типа того

private void CreateRelation() {
// Get the DataColumn objects from two DataTable objects in a DataSet.
DataColumn parentCol;
DataColumn childCol;
// Code to get the DataSet not shown here.
parentCol = DataSet1.Tables["Customers"].Columns["CustID"];
childCol = DataSet1.Tables["Orders"].Columns["CustID"];
// Create DataRelation.
DataRelation relCustOrder;
relCustOrder = new DataRelation("CustomersOrders", parentCol, childCol);
// Add the relation to the DataSet.
DataSet1.Relations.Add(relCustOrder);